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The text summarizes selected chapters from my dissertation thesis which was awarded by the 2016 European Photochemistry Association PhD Prize. It reports on the development of first fully-organic visible light absorbing photoremovable protecting group and carbon-monoxide releasing compounds. These dye-based molecules were rationally designed, carefully synthetized and their properties were investigated in detail. Some of them were also used for in vivo and in vitro biological studies.

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