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Nanoscience & Nanotechnology Series
Nanostructured Catalysts: Selective Oxidations
By
Royal Society of Chemistry
Royal Society of Chemistry
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Edited by
Christian Hess;
Christian Hess
Eduard-Zintl-Institut für Anorganische Chemie und Physikalische Chemie, Germany
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Robert Schlögl
Robert Schlögl
Fritz Haber Institute of the Max Planck Society, Germany
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Hardback ISBN:
978-0-85404-186-2
PDF ISBN:
978-1-84755-987-6
Special Collection:
2011 ebook collection
,
2011 ebook collection
,
2011-2015 physical chemistry subject collection
Series:
Nanoscience & Nanotechnology
No. of Pages:
452
Published online:
22 Jul 2011
Published in print:
09 Aug 2011
Book Chapter
Chapter 2: C–H Activation of Alkanes in Selective Oxidation Reactions on Solid Oxide Catalysts
By
Johannes A. Lercher
;
Johannes A. Lercher
Technische Universität München, Department of Chemistry and Catalysis Research Center
Lichtenbergstraße 4
85747
Garching
Germany
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Frederik N. Naraschewski
Frederik N. Naraschewski
Technische Universität München, Department of Chemistry and Catalysis Research Center
Lichtenbergstraße 4
85747
Garching
Germany
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-
Published:22 Jul 2011
-
Special Collection: 2011 ebook collection , 2011 ebook collection , 2011-2015 physical chemistry subject collectionSeries: Nanoscience & Nanotechnology
Page range:
5 - 32
Citation
J. A. Lercher and F. N. Naraschewski, in Nanostructured Catalysts: Selective Oxidations, ed. C. Hess and R. Schlögl, The Royal Society of Chemistry, 2011, ch. 2, pp. 5-32.
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This chapter is focused on the initial activation step of C–H bonds in oxidation reactions. Model experiments, kinetic analysis of complex reactions and theoretical studies will be combined to provide an overview on the current state of insight into the processes as well as their potentials and limitations. The chapter covers processes on oxide clusters, indirect oxidation via electrophilic substitution reactions (chlorination and bromination) and the influence of anions and nonreducible cations on the mechanism of C–H activation.
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