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This solid-state NMR report summarises the subject and results of 250 articles and original papers published in 2021. In addition to the published reviews, the two major sections in this report consider various methodological developments and a broad range of applications. The presented classification of papers into different sections and subsections is intended to ease the overview of the results obtained in 2021, as well as to evaluate the directions in which solid-state NMR techniques and applications are likely to develop in the near future.

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