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Green Chemistry Series
Chemical Valorisation of Carbon Dioxide
Edited by
Georgios Stefanidis;
Georgios Stefanidis
National Technical University of Athens, Greece and University of Ghent, Belgium
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Andrzej Stankiewicz
Andrzej Stankiewicz
Delft University of Technology, The Netherlands
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Hardback ISBN:
978-1-83916-407-1
PDF ISBN:
978-1-83916-764-5
EPUB ISBN:
978-1-83916-765-2
Special Collection:
2022 ebook collection
Series:
Green Chemistry
No. of Pages:
564
Publication date:
19 Dec 2022
Book Chapter
Chapter 5: Homogeneous CO2 Hydrogenation
By
J. Ferrer
;
J. Ferrer
Instituto de Síntesis Química y Catálisis Homogénea, Consejo Superior de Investigaciones Científicas-Universidad de Zaragoza, Departamento de Química Inorgánica
Pedro Cerbuna 12
50009 Zaragoza
Spain
dcarmona@unizar.es
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V. Passarelli
;
V. Passarelli
Instituto de Síntesis Química y Catálisis Homogénea, Consejo Superior de Investigaciones Científicas-Universidad de Zaragoza, Departamento de Química Inorgánica
Pedro Cerbuna 12
50009 Zaragoza
Spain
dcarmona@unizar.es
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D. Carmona
D. Carmona
Instituto de Síntesis Química y Catálisis Homogénea, Consejo Superior de Investigaciones Científicas-Universidad de Zaragoza, Departamento de Química Inorgánica
Pedro Cerbuna 12
50009 Zaragoza
Spain
dcarmona@unizar.es
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Published:19 Dec 2022
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Special Collection: 2022 ebook collectionSeries: Green Chemistry
Citation
J. Ferrer, V. Passarelli, and D. Carmona, in Chemical Valorisation of Carbon Dioxide, ed. G. Stefanidis and A. Stankiewicz, The Royal Society of Chemistry, 2022, ch. 5, pp. 97-127.
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This contribution will focus on the hydrogenation of carbon dioxide to formic acid or methanol using homogeneous catalysts, mostly transition metal complexes, and molecular dihydrogen as the reductant. Homogeneously catalysed indirect reduction of carbon dioxide via hydrogenation of intermediates such as formamides, carbonates, carbamates and ureas is also considered. The proposed mechanisms for these transformations are revised.
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