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Conductive metal–organic frameworks (C-MOFs), also known as smart intrinsically porous extended materials, have attracted enormous attention in the research community. C-MOFs have attracted enormous attention from the research community due to their intrinsic conductivity, numerous active sites, and chemical and thermal stability, making them useful in a wide range of applications, including sensors. C-MOF-based sensors mainly fall into two categories: chemiresistive sensors and electrochemical sensors. This chapter describes C-MOFs, their synthesis procedure, and their use as active materials for developing and designing sensors.

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