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This chapter points out the main challenges of using anisotropic NMR parameters for organic structure elucidation and also where differences to biomolecular applications lie. The challenges include the necessity of determining configurations and conformations at the same time, the diverse and extended spin-systems present in organic compounds and the necessity of using organic solvents. The chapter aims at providing an overview of the most recent solutions to these challenges and which opportunities there are if one uses anisotropic NMR parameters for structure elucidation of organic compounds.

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