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Metallosupramolecular materials incorporating spin-crossover (SCO) properties are a rapidly expanding field of advanced materials research. Discrete species are a target for their fundamental interest as prototypes of infinite polymeric materials and for their unique SCO properties. At this time, a heptanuclear material is the highest nuclearity discrete SCO species reported. Greater nuclearities are sought for their “nano-sized” dimensions representative of the “bottom-up” approach to nano-complexes. Polymeric species are important for their cooperative SCO properties and advanced multi-functional features.

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