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Metal–organic frameworks (MOFs) represent a fascinating class of porous crystalline materials due to their designable pore structure and functionality. MOF/polymer hybrid membranes, taking advantage of the molecular sieving property of MOFs and good processability of polymers, have been gradually becoming the next-generation competitive membrane materials. Recent years have witnessed significant progress in MOF/polymer composite membranes. In this chapter, we discuss opportunities and challenges related to the rational design of MOF/polymer composite membranes including MOF-based mixed matrix membranes (MMMs) and polymer-supported MOF membranes. We also highlight their latest application progress in the area of liquid separations such as water treatment, organic solvent nanofiltration and pervaporation, along with gas separations.

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